The rare-earth triangular-lattice chalcogenide is a great platform for exploring both spin liquids and novel magnetic orders with anisotropic spin interactions and magnetic frustrations. Here, we report the thermodynamic and neutron scattering measurements of rare-earth triangular-lattice chalcogenide KErSe2, using single-crystal samples. Our experiments revealed a long-range stripe order below 0.2 K. Although the magnetic order was three-dimensional, magnetic excitations exhibited negligible modulation along the z direction, indicating very weak interlayer coupling. Furthermore, magnetic excitation developed a well-defined spin-wave dispersion with a gap of ∼0.03 meV at M points. Both the stripe order and spin-wave excitations could be quantitatively understood from the anisotropic spin interactions of the Er3+ Kramers doublets.
@article{arxiv.2210.15867,
title = {Stripe order and spin dynamics in triangular-lattice antiferromagnet KErSe$_{2}$: A single-crystal study with a theoretical description},
author = {Gaofeng Ding and Hongliang Wo and Rui Leonard Luo and Yimeng Gu and Yiqing Gu and Robert Bewley and Gang Chen and Jun Zhao},
journal= {arXiv preprint arXiv:2210.15867},
year = {2023}
}