English

Strain-induced structural change and nearly-commensurate diffuse scattering in the model high-temperature superconductor HgBa$_2$CuO$_{4+\delta}$

Superconductivity 2026-04-24 v1

Abstract

We investigate the strain response of underdoped HgBa2_2CuO4+δ_{4+\delta} (Hg1201), by synchrotron X-ray diffraction and corresponding simulations of thermal diffuse scattering. The compression in the crystallographic aa direction leads to relatively small expansion in the bb and cc directions, with Poisson ratios νba\nu_{ba}=0.16 and νca\nu_{ca}=0.11, respectively. However, the Cu-O distance in the cc direction exhibits a notable 0.9% increase at 1.1% aa-axis compression. We further find strain-induced diffuse scattering which corresponds to a new type of two-dimensional charge correlation. Interestingly, this signal is insensitive to the onset of superconductivity and instead corresponds to a short-range, nearly commensurate modulation with a wave vector close to (0.5, 0, 0) and a correlation length of approximately four unit cells. It closely resembles the charge order theoretically predicted in the phase diagram of the spin-liquid model with resonating valence bonds on a square lattice.

Keywords

Cite

@article{arxiv.2510.21343,
  title  = {Strain-induced structural change and nearly-commensurate diffuse scattering in the model high-temperature superconductor HgBa$_2$CuO$_{4+\delta}$},
  author = {Mai Ye and Wenshan Hong and Tom Lacmann and Mehdi Frachet and Igor Vinograd and Gaston Garbarino and Sofia-Michaela Souliou and Michael Merz and Rolf Heid and Amir-Abbas Haghighirad and Yuan Li and Matthieu Le Tacon},
  journal= {arXiv preprint arXiv:2510.21343},
  year   = {2026}
}