We report on the magnetic properties of geometrically frustrated K3CrO4, in which Cr5+ cations are arranged on a distorted pyrochlore lattice. The crystal structure, static and dynamic magnetic properties of the compound are investigated in detail. A combination of DC and AC magnetic susceptibility measurements together with thermoremanent magnetization decay measurements reveal several magnetic transitions: the onset of glassy canted antiferromagnetic order occurs at 36 K, followed by the appearance of ferromagnetic/ferrimagnetic cluster glass behavior below the freezing temperature of 20 K. Further field-induced, temperature-dependent transitions are observed in the range 3-10 K. The frequency dependence of the freezing temperature for the cluster glass state is analyzed on the basis of dynamic scaling laws including the critical slowing down formula and the Vogel-Fulcher law.
@article{arxiv.2107.02878,
title = {Static and dynamic magnetic properties of K3CrO4},
author = {Liliia D. Kulish and Graeme R. Blake},
journal= {arXiv preprint arXiv:2107.02878},
year = {2021}
}
Comments
A high-resolution version with supplementary material can be found at https://www.sciencedirect.com/science/article/pii/S0304885321004893?via%3Dihub. arXiv admin note: text overlap with arXiv:1912.05997