Stacking-dependent anisotropic altermagnetism in V$_{1/3}$NbS$_2$
Abstract
We report profound impacts of the stacking sequence of triangular lattices of magnetic transition metal ions intercalated between the layers of the van der Waals material NbS. Using single crystal x-ray and neutron diffraction, and transport and magnetization measurements, we show there are two distinct polytypes of with disparate easy axes of magnetization and different anomalous Hall responses. Self-consistent analysis of inelastic neutron scattering data provides evidence for oscillatory RKKY interactions that extend to 1 nm and stabilize quasi-collinear A-type altermagnetic orders in both polytypes though with perpendicular easy axes. The detailed stacking sequence of a bulk polytype crystal dramatically impact its macroscopic anomalous Hall response and magnetism, which suggests a new path to engineer the bulk properties of a layered three dimensional solid.
Cite
@article{arxiv.2607.25213,
title = {Stacking-dependent anisotropic altermagnetism in V$_{1/3}$NbS$_2$},
author = {Chris J. Lygouras and Nathan Prouse and Jack H. Drouin and Youzhe Chen and Laura Garcia-Gassull and Zili Feng and Mingxuan Fu and Lü Fang and Alexander I. Kolesnikov and Christina Hoffman and Yiqing Hao and Huibo Cao and Maxime A. Siegler and Robert J. Birgeneau and Roser Valentí and Satoru Nakatsuji and Collin L. Broholm},
journal= {arXiv preprint arXiv:2607.25213},
year = {2026}
}
Comments
9 pages manuscript plus 11 pages SI, 16 figures