Spin excitations in a single La$_2$CuO$_4$ layer
Abstract
The dynamics of S=1/2 quantum spins on a 2D square lattice lie at the heart of the mystery of the cuprates \cite{Hayden2004,Vignolle2007,Li2010,LeTacon2011,Coldea2001,Headings2010,Braicovich2010}. In bulk cuprates such as \LCO{}, the presence of a weak interlayer coupling stabilizes 3D N\'{e}el order up to high temperatures. In a truly 2D system however, thermal spin fluctuations melt long range order at any finite temperature \cite{Mermin1966}. Further, quantum spin fluctuations transfer magnetic spectral weight out of a well-defined magnon excitation into a magnetic continuum, the nature of which remains controversial \cite{Sandvik2001,Ho2001,Christensen2007,Headings2010}. Here, we measure the spin response of \emph{isolated one-unit-cell thick layers} of \LCO{}. We show that coherent magnons persist even in a single layer of \LCO{} despite the loss of magnetic order, with no evidence for resonating valence bond (RVB)-like spin correlations \cite{Anderson1987,Hsu1990,Christensen2007}. Thus these excitations are well described by linear spin wave theory (LSWT). We also observe a high-energy magnetic continuum in the isotropic magnetic response. This high-energy continuum is not well described by 2 magnon LSWT, or indeed any existing theories.
Cite
@article{arxiv.1208.0018,
title = {Spin excitations in a single La$_2$CuO$_4$ layer},
author = {M. P. M. Dean and R. S. Springell and C. Monney and K. J. Zhou and I. Bozovic and J. Pereiro and B. Dalla Piazza and H. M. Ronnow and E. Morenzoni and J. van den Brink and T. Schmitt and J. P. Hill},
journal= {arXiv preprint arXiv:1208.0018},
year = {2012}
}
Comments
Revised version to appear in Nature Materials; 6 pages,4 figures