English

Speed limits of the laser-induced phase transition in FeRh

Materials Science 2024-11-11 v4

Abstract

We use ultrafast x-ray diffraction (UXRD) and the polar time-resolved magneto-optical Kerr effect (tr-MOKE) to study the laser-induced metamagnetic phase transition in two FeRh films with thicknesses below and above the optical penetration depth. In the thin film, we identify an intrinsic timescale for the light-induced nucleation of ferromagnetic (FM) domains in the antiferromagnetic material of 8ps8\,\text{ps} that is substantially slower than the speed of sound. For the inhomogeneously excited thicker film, only the optically excited near-surface part transforms within 8ps8\,\text{ps}. For strong excitations we observe an additional slow rise of the FM phase, which we experimentally relate to a growth of the FM phase into the depth of the layer by comparing the transient magnetization in front- and backside excitation geometry. In the lower lying parts of the film, which are only excited via near-equilibrium heat transport, the FM phase emerges significantly slower than 8ps8\,\text{ps} after heating above the transition temperature.

Keywords

Cite

@article{arxiv.2305.02094,
  title  = {Speed limits of the laser-induced phase transition in FeRh},
  author = {Maximilian Mattern and Jasmin Jarecki and Jon Ander Arregi and Vojtěch Uhlíř and Matthias Rössle and Matias Bargheer},
  journal= {arXiv preprint arXiv:2305.02094},
  year   = {2024}
}