We use ultrafast x-ray diffraction (UXRD) and the polar time-resolved magneto-optical Kerr effect (tr-MOKE) to study the laser-induced metamagnetic phase transition in two FeRh films with thicknesses below and above the optical penetration depth. In the thin film, we identify an intrinsic timescale for the light-induced nucleation of ferromagnetic (FM) domains in the antiferromagnetic material of 8ps that is substantially slower than the speed of sound. For the inhomogeneously excited thicker film, only the optically excited near-surface part transforms within 8ps. For strong excitations we observe an additional slow rise of the FM phase, which we experimentally relate to a growth of the FM phase into the depth of the layer by comparing the transient magnetization in front- and backside excitation geometry. In the lower lying parts of the film, which are only excited via near-equilibrium heat transport, the FM phase emerges significantly slower than 8ps after heating above the transition temperature.
@article{arxiv.2305.02094,
title = {Speed limits of the laser-induced phase transition in FeRh},
author = {Maximilian Mattern and Jasmin Jarecki and Jon Ander Arregi and Vojtěch Uhlíř and Matthias Rössle and Matias Bargheer},
journal= {arXiv preprint arXiv:2305.02094},
year = {2024}
}