English

Solvent-triggered shape change in gradient-based 4D printed bilayers: case study on semi-crystalline polymer networks

Soft Condensed Matter 2025-01-09 v1 Materials Science

Abstract

We propose an approach to 4D print solvent-triggered, gradient-based bilayers made of semi-crystalline crosslinked polymer networks. Out-of-plane bending is obtained after immersion in the solvent, exploiting the different swelling degrees of the layers resulting from crosslinking gradients. Lastly, a beam model of the shape transformation is applied and experimentally validated.

Cite

@article{arxiv.2501.04546,
  title  = {Solvent-triggered shape change in gradient-based 4D printed bilayers: case study on semi-crystalline polymer networks},
  author = {Lorenzo Bonetti and Aron Cobianchi and Daniele Natali and Stefano Pandini and Massimo Messori and Maurizio Toselli and Giulia Scalet},
  journal= {arXiv preprint arXiv:2501.04546},
  year   = {2025}
}

Comments

This work was funded by the European Union ERC CoDe4Bio Grant ID 101039467 under the funding programme Horizon Europe

R2 v1 2026-06-28T20:59:55.364Z