Soft X-ray imaging with coherence tomography in the water window spectral range using high-harmonic generation
Abstract
High-harmonic generation (HHG) is used as a source for various imaging applications in the extreme ultraviolet spectral range. It offers spatially coherent radiation and unique elemental contrast with the potential for attosecond time resolution. The unfavorable efficiency scaling to higher photon energies prevented the imaging application in the soft X-ray range so far. In this work we demonstrate the feasibility of using harmonics for imaging in the water window spectral region (284eV to 532eV). We achieve nondestructive depth profile imaging in a heterostructure by utilizing a broadband and noise-resistant technique called soft X-ray Coherence Tomography (SXCT) at a high-flux lab-scale HHG source. SXCT is derived from Optical Coherence Tomography, a Fourier based technique, that can use the full bandwidth of the source to reach an axial resolution of 12nm in this demonstration. The employed source covers the entire water window, with a photon flux exceeding 10photons/eV/s at a photon energy of 500eV. We show local cross sections of a sample consisting of Aluminium oxide and Platinum layers of varying thickness on a Zinc oxide substrate. We validate the findings with scanning and transmission electron microscopy after preparation with focused ion beam milling.
Cite
@article{arxiv.2503.04276,
title = {Soft X-ray imaging with coherence tomography in the water window spectral range using high-harmonic generation},
author = {Julius Reinhard and Felix Wiesner and Themistoklis Sidiropoulos and Martin Hennecke and Sophia Kaleta and Julian Späthe and Johann Jakob Abel and Martin Wünsche and Gabriele Schmidl and Jonathan Plentz and Uwe Hübner and Katharina Freiberg and Jonathan Apell and Stephanie Lippmann and Matthias Schnürer and Stefan Eisebitt and Gerhard G. Paulus and Silvio Fuchs},
journal= {arXiv preprint arXiv:2503.04276},
year = {2025}
}
Comments
9 pages, 4 figures, preprint