Shear Flows and Segregation in the Reaction $A+B\to\emptyset$
Abstract
We study theoretically and numerically the effects of the linear velocity field on the irreversible reaction . Assuming homogeneous initial conditions for the two species, with equal initial densities, we demonstrate the presence of a crossover time . For , the kinetics are unaffected by the shear and we retain both the effect of species segregation (for ) and the density decay rate , where . We calculate the amplitude to leading order in a small density expansion for , and give bounds in . However, for , the critical dimension for anomalous kinetics is reduced to , with the density decay rate holding for . Bounds are calculated for the amplitude in , which depend on the velocity gradient and the (equal) diffusion constants . We also briefly consider the case of a non-linear shear flow, where we give a more general form for the crossover time . Finally, we perform numerical simulations for a linear shear flow in with results in agreement with theoretical predictions.
Keywords
Cite
@article{arxiv.cond-mat/9601098,
title = {Shear Flows and Segregation in the Reaction $A+B\to\emptyset$},
author = {M. J. Howard and G. T. Barkema},
journal= {arXiv preprint arXiv:cond-mat/9601098},
year = {2009}
}
Comments
26 pages latex document, 13 figures, uses epsf.sty