English

Self-motility of an active particle induced by correlations in the surrounding solution

Soft Condensed Matter 2021-01-01 v1 Chemical Physics

Abstract

Current models of phoretic transport rely on molecular forces creating a "diffuse" particle-fluid interface. We investigate theoretically an alternative mechanism, in which a diffuse interface emerges solely due to a non-vanishing correlation length of the surrounding solution. This mechanism can drive self-motility of a chemically active particle. Numerical estimates indicate that the velocity can reach micrometers per second. The predicted phenomenology includes a bilinear dependence of the velocity on the activity and a possible double velocity reversal upon varying the correlation length.

Keywords

Cite

@article{arxiv.2011.02528,
  title  = {Self-motility of an active particle induced by correlations in the surrounding solution},
  author = {Alvaro Domínguez and M. N. Popescu and C. M. Rohwer and S. Dietrich},
  journal= {arXiv preprint arXiv:2011.02528},
  year   = {2021}
}

Comments

6 pages, 2 figures, and 22 pages of supplemental material. To be published as Phys. Rev. Lett