English

Self-induced spin glass state in elemental and crystalline neodymium

Materials Science 2020-06-01 v2 Statistical Mechanics

Abstract

Spin glasses are a highly complex magnetic state of matter, intricately linked to spin frustration and structural disorder. They exhibit no long-range order and exude aging phenomena, distinguishing them from quantum spin liquids. We report a new type of spin glass state, the spin-Q glass, observable in bulk-like crystalline metallic neodymium thick films. Using spin-polarized scanning tunneling microscopy combined with ab initio calculations and atomistic spin-dynamics simulations, we visualize the variations in atomic-scale non-collinear order and its response to magnetic field and temperature. We quantify the aging phenomena relating the glassiness to crystalline symmetry and the energy landscape. This result not only resolves the long-standing debate of the magnetism of neodymium, but also suggests that glassiness may arise in other magnetic solids lacking extrinsic disorder.

Keywords

Cite

@article{arxiv.1907.02295,
  title  = {Self-induced spin glass state in elemental and crystalline neodymium},
  author = {Umut Kamber and Anders Bergman and Andreas Eich and Diana Iuşan and Manuel Steinbrecher and Nadine Hauptmann and Lars Nordström and Mikhail I. Katsnelson and Daniel Wegner and Olle Eriksson and Alexander A. Khajetoorians},
  journal= {arXiv preprint arXiv:1907.02295},
  year   = {2020}
}