English

Scaling and data collapse from local moments in frustrated disordered quantum spin systems

Strongly Correlated Electrons 2018-10-23 v3 Disordered Systems and Neural Networks

Abstract

Recently measurements on various spin-1/2 quantum magnets such as H3_3LiIr2_2O6_6, LiZn2_2Mo3_3O8_8, ZnCu3_3(OH)6_6Cl2_2 and 1T-TaS2_2 -- all described by magnetic frustration and quenched disorder but with no other common relation -- nevertheless showed apparently universal scaling features at low temperature. In particular the heat capacity C[H,T] in temperature T and magnetic field H exhibits T/H data collapse reminiscent of scaling near a critical point. Here we propose a theory for this scaling collapse based on an emergent random-singlet regime extended to include spin-orbit coupling and antisymmetric Dzyaloshinskii-Moriya (DM) interactions. We derive the scaling C[H,T]/THγFq[T/H]C[H,T]/T \sim H^{-\gamma} F_q[T/H] with Fq[x]=xqF_q[x] = x^{q} at small xx, with qq \in (0,1,2) an integer exponent whose value depends on spatial symmetries. The agreement with experiments indicates that a fraction of spins form random valence bonds and that these are surrounded by a quantum paramagnetic phase. We also discuss distinct scaling for magnetization with a qq-dependent subdominant term enforced by Maxwell's relations.

Keywords

Cite

@article{arxiv.1803.00013,
  title  = {Scaling and data collapse from local moments in frustrated disordered quantum spin systems},
  author = {Itamar Kimchi and John P. Sheckelton and Tyrel M. McQueen and Patrick A. Lee},
  journal= {arXiv preprint arXiv:1803.00013},
  year   = {2018}
}

Comments

v2. Expanded argument in Appendix 2 and revised for clarity. v3. Fixed typo in Fig 3 caption. Main text 4 pages 4 figures, Appendix 6 pages 1 figure

R2 v1 2026-06-23T00:37:13.829Z