The discovery of the nonlinear Hall effect provides an avenue for studying the interplay among symmetry, topology, and phase transitions, with potential applications in signal doubling and high-frequency rectification. However, practical applications require devices fabricated on large area thin film as well as room-temperature operation. Here, we demonstrate robust room-temperature nonlinear transverse response and microwave rectification in MnBi2Te4 films grown by molecular beam epitaxy. We observe multiple sign-reversals in the nonlinear response by tuning the chemical potential. Through theoretical analysis, we identify skew scattering and side jump, arising from extrinsic spin-orbit scattering, as the main mechanisms underlying the observed nonlinear signals. Furthermore, we demonstrate radio frequency (RF) rectification in the range of 1-8 gigahertz at 300 K. These findings not only enhance our understanding of the relationship between nonlinear response and magnetism, but also expand the potential applications as energy harvesters and detectors in high-frequency scenarios.
@article{arxiv.2412.15591,
title = {Room-temperature nonlinear transport and microwave rectification in antiferromagnetic MnBi$_2$Te$_4$ films},
author = {Shanshan Liu and Rhonald Burgos and Enze Zhang and Naizhou Wang and Xiao-Bin Qiang and Chuanzhao Li and Qihan Zhang and Z. Z. Du and Rui Zheng and Jingsheng Chen and Qing-Hua Xu and Kai Leng and Weibo Gao and Faxian Xiu and Dimitrie Culcer and Kian Ping Loh},
journal= {arXiv preprint arXiv:2412.15591},
year = {2024}
}