English

RKKY-dipolar Interactions and 3D Spin Supersolid on Stacked Triangular Lattice

Strongly Correlated Electrons 2026-03-26 v1

Abstract

Inspired by the recent discovery of metallic spin supersolidity and its giant magnetocaloric effect in the rare-earth alloy EuCo2_2Al9_9 [Nature 651, 61 (2026)], we perform a combined study through electronic structure analysis, effective spin model, and Monte Carlo simulations on a stacked triangular lattice, and reveal a novel mechanism for the emergence of 3D spin supersolid in a metallic antiferromagnet. From first-principles inputs, we derive a minimal spin model on a stacked triangular lattice (STL), which arises from the interplay between Ruderman-Kittel-Kasuya-Yosida (RKKY) and dipolar interactions and accurately reproduces the experimental thermodynamics. Based on the STL model, we identify a ground state that simultaneously breaks discrete lattice translational symmetry and continuous spin-rotational symmetry -- the hallmark of a spin supersolid. Furthermore, we present the field-temperature phase diagram of the 3D STL model and discuss the various magnetic phases and associated phase transitions. Under zero field, the spin supersolid Y order establishes in two steps: an upper transition at TN1T_{N1}, where an emergent U(1) symmetry appears and the system enters a fluctuating collinear regime, followed by a lower transition at TN2T_{N2} into the spin supersolid Y phase. In contrast, the supersolid V phase undergoes a single phase transition at TNVT_N^V. Our results not only provide a comprehensive theoretical understanding of the metallic spin supersolid reported for EuCo2_2Al9_9 but also pave the way for further experimental investigations into its supersolid transitions and universality class.

Keywords

Cite

@article{arxiv.2603.24446,
  title  = {RKKY-dipolar Interactions and 3D Spin Supersolid on Stacked Triangular Lattice},
  author = {Ning Xi and Xitong Xu and Guoliang Wu and Mingfang Shu and Hao Chen and Yuan Gao and Zhentao Wang and Gang Su and Jie Ma and Zhe Qu and Xi Chen and Wei Li},
  journal= {arXiv preprint arXiv:2603.24446},
  year   = {2026}
}

Comments

9 pages, 5 figures

R2 v1 2026-07-01T11:37:31.798Z