English

Resonant thermoelectric transport in atomic chains with Fano defects

Mesoscale and Nanoscale Physics 2018-06-08 v1 Materials Science

Abstract

Atomic clusters attached to a low-dimensional system, called Fano defects, produce rich wave interferences. In this work, we analytically found an enhanced thermoelectric figure-of-merit (ZT) in periodic atomic chains with Fano defects, compared to those without such defects. We further study self-assembled DNA-like systems with periodic and quasiperiodically placed Fano defects by using a real-space renormalization method developed for the Kubo-Greenwood formula, in which tight-binding and Born models are respectively used for the electric and lattice thermal conductivities. The results reveal that the quasiperiodicity could be another ZT-improving factor, whose long-range disorder inhibits low-frequency acoustic phonons insensitive to local defects.

Keywords

Cite

@article{arxiv.1805.02271,
  title  = {Resonant thermoelectric transport in atomic chains with Fano defects},
  author = {J. Eduardo González and Vicenta Sánchez and Chumin Wang},
  journal= {arXiv preprint arXiv:1805.02271},
  year   = {2018}
}

Comments

Accepted version in MRS Communications