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Quasiparticle bandstructure effects on the {\it d} hole lifetimes of copper within the GW approximation

Strongly Correlated Electrons 2009-11-07 v1 Materials Science

Abstract

We investigate the lifetime of {\it d} holes in copper within a {\it first--principle} GWGW approximation. At the G0W0G_0W_0 level the lifetime of the topmost {\it d} bands are in agreement with the experimental results and are four times smaller than those obtained in the ``on--shell'' calculations commonly used in literature. The theoretical lifetimes and bandstructure, however, worsen when further iterative steps of self-consistency are included in the calculation, pointing to a delicate interplay between self--consistency and the inclusion of vertex corrections. We show that the G0W0G_0W_0 success in the lifetimes calculation is due to the opening of new ``intraband'' decay channels that disappear at self--consistency.

Keywords

Cite

@article{arxiv.cond-mat/0208575,
  title  = {Quasiparticle bandstructure effects on the {\it d} hole lifetimes of copper within the GW approximation},
  author = {Andrea Marini and Rodolfo Del Sole and Angel Rubio and Giovanni Onida},
  journal= {arXiv preprint arXiv:cond-mat/0208575},
  year   = {2009}
}

Comments

Accepted for pubblication on Physical Review B, Rapid Communications