English

Polydisperse Adsorption: Pattern Formation Kinetics, Fractal Properties, and Transition to Order

Statistical Mechanics 2009-10-31 v1 Disordered Systems and Neural Networks Soft Condensed Matter

Abstract

We investigate the process of random sequential adsorption of polydisperse particles whose size distribution exhibits a power-law dependence in the small size limit, P(R)Rα1P(R)\sim R^{\alpha-1}. We reveal a relation between pattern formation kinetics and structural properties of arising patterns. We propose a mean-field theory which provides a fair description for sufficiently small α\alpha. When α\alpha \to \infty, highly ordered structures locally identical to the Apollonian packing are formed. We introduce a quantitative criterion of the regularity of the pattern formation process. When α1\alpha \gg 1, a sharp transition from irregular to regular pattern formation regime is found to occur near the jamming coverage of standard random sequential adsorption with monodisperse size distribution.

Keywords

Cite

@article{arxiv.cond-mat/9806331,
  title  = {Polydisperse Adsorption: Pattern Formation Kinetics, Fractal Properties, and Transition to Order},
  author = {N. V. Brilliantov and Yu. A. Andrienko and P. L. Krapivsky and J. Kurths},
  journal= {arXiv preprint arXiv:cond-mat/9806331},
  year   = {2009}
}

Comments

8 pages, LaTeX, 5 figures, to appear in Phys.Rev.E