English

Polar phase transition in $180^{\circ}$-domain wall of lead titanate

Materials Science 2022-10-04 v1

Abstract

A new mechanism leading to a switchable polarization in a ferroelectric domain wall (DW) is proposed. A biquadratic coupling of the primary order parameter and its gradient triggers the phase transition in the DW with softening of the local polar mode and anomalous increase of the susceptibility at the phase transition temperature TDWT_{DW}. This mechanism describes the origin and properties of the polar Bloch and antipolar N\'eel components in the 180180^\circ-DW of PbTiO3_3, which were recently reported from first-principles calculations.

Keywords

Cite

@article{arxiv.2210.00793,
  title  = {Polar phase transition in $180^{\circ}$-domain wall of lead titanate},
  author = {I. Rychetsky and W. Schranz and A. Tröster},
  journal= {arXiv preprint arXiv:2210.00793},
  year   = {2022}
}

Comments

5 pages, 4 PDF figures