English

Photoinduced melting dynamics and collective mode in a correlated charge-ordered system

Strongly Correlated Electrons 2026-03-19 v2

Abstract

We theoretically investigate the transient spectral function during the photoinduced melting of charge order in a correlated electron system, to unravel the dynamical processes triggered by different initial excitations. We employ a one-dimensional interacting spinless fermion model introducing a pulsed laser light, and perform a comparative study by the Hartree-Fock approximation and by the exact diagonalization method to numerically solve the time-dependent Schr\"odinger equation. We find characteristic behavior in the transient spectral function, whose features strongly depend on the pump light frequency ωp\omega_p. When ωp\omega_p is resonant with the collective phase mode of frequency ΩcΔCO/2\Omega_c\simeq \Delta_{\rm CO}/2, where ΔCO\Delta_{\rm CO} is the charge gap, the transient spectral function exhibits a photoinduced in-gap weight which triggers large responses. With increasing the laser intensity, the development of in-gap weight directly turns into the collapse of the gap. This charge-order destabilization process is in sharp contrast to the case of ωp>ΔCO\omega_p>\Delta_{\rm CO}, where the photoirradiation induces interband electron-hole excitations giving rise to a shrinkage of the gap. The impact of quantum fluctuations and spatial inhomogeneity on the photoinduced dynamics is also discussed.

Keywords

Cite

@article{arxiv.2510.16855,
  title  = {Photoinduced melting dynamics and collective mode in a correlated charge-ordered system},
  author = {Yasuhiro Tanaka and Hitoshi Seo},
  journal= {arXiv preprint arXiv:2510.16855},
  year   = {2026}
}

Comments

10 pages, 12 figures, to be published in Phys. Rev. B