English

Phase transformations in methanol at high pressure measured by dielectric spectroscopy technique

Materials Science 2015-06-15 v2 Soft Condensed Matter

Abstract

Dielectric response in methanol measured in wide pressure and temperature range (P<6.0P < 6.0 GPa; 100 K <T<<T< 360 K) reveals a series of anomalies which can be interpreted as a transformation between several solid phases of methanol including a hitherto unknown high-pressure low-temperature phase with stability range P>P > 1.2 GPa T<270T < 270 K. In the intermediate P-T region P3.43.7P \approx 3.4-3.7 GPa T260280T \approx 260-280 K a set of complicated structural transformations occurs involving four methanol crystalline structures. At higher pressures within a narrow range P4.34.5P \approx 4.3-4.5 GPa methanol can be obtained in the form of fragile glass (Tg200T_g \approx 200 K, mp80m_p \approx 80 at P=4.5P= 4.5 GPa) by relatively slow cooling.

Keywords

Cite

@article{arxiv.1305.3171,
  title  = {Phase transformations in methanol at high pressure measured by dielectric spectroscopy technique},
  author = {M. V. Kondrin and A. A. Pronin and Y. B. Lebed and V. V. Brazhkin},
  journal= {arXiv preprint arXiv:1305.3171},
  year   = {2015}
}

Comments

Submitted to JCP