English

Permutation invariant multi-scale full quantum neural network wavefunction

Chemical Physics 2026-03-13 v1

Abstract

Solving the intricate quantum behavior of interacting particles is key to unlocking the mysteries of condensed matter, but capturing their complex correlations across different scales remains a monumental challenge. We introduce a neural network framework that overcomes this barrier by modeling the full quantum wavefunction of a system, including electrons, nuclei and muons, directly capturing the full quantum effects beyond the Born-Oppenheimer approximation. The neural network approximates joint wavefunction of different interacting particles with a rigorous handling of permutation invariance, enabling simultaneous treatment of nuclear quantum effects and electron-nucleus-muon couplings without explicit excited states. Validated on molecular systems, this approach offers a computationally feasible way to model full quantum phenomena in complex many-body systems, establishing a direct connection between fundamental particle properties and emergent material behavior.

Keywords

Cite

@article{arxiv.2603.12233,
  title  = {Permutation invariant multi-scale full quantum neural network wavefunction},
  author = {Pengzhen Cai and Yubing Qian and Li Deng and Weizhong Fu and Lei Yang and Zhiyu Sun and Xin-Zheng Li and En-Ge Wang and Liangwen Chen and Weiluo Ren and Ji Chen},
  journal= {arXiv preprint arXiv:2603.12233},
  year   = {2026}
}