English

Paramagnon dispersion and damping in doped Na$_{x}$Ca$_{2-x}$CuO$_2$Cl$_2$

Superconductivity 2023-07-13 v6 Strongly Correlated Electrons

Abstract

Using Resonant Inelastic X-ray Scattering, we measure the paramagnon dispersion and damping of undoped, antiferromagnetic Ca2_2CuO2_2Cl2_2 as well as doped, superconducting Nax_{x}Ca2x_{2-x}CuO2_2Cl2_2. Our estimation of the spin-exchange parameter and width of the paramagnon peak at the zone boundary X=(0.5,0)X=(0.5,0) confirms that no simple relation can be drawn between these parameters and the critical temperature TcT_\mathrm{c}. Consistently with other cuprate compounds, we show that upon doping there is a slight softening at (0.25,0)(0.25,0), but not at the zone boundary XX. In combination with these measurements we perform calculations of the dynamical spin structure factor of the one-band Hubbard model using cluster dynamical mean-field theory. The calculations are in excellent agreement with the experiment in the undoped case, both in terms of energy position and width. While the increase in width is also captured upon doping, the dynamical spin structure factor shows a sizable softening at XX, which provides insightful information on the length-scale of the spin fluctuations in doped cuprates.

Keywords

Cite

@article{arxiv.2303.04139,
  title  = {Paramagnon dispersion and damping in doped Na$_{x}$Ca$_{2-x}$CuO$_2$Cl$_2$},
  author = {Blair W. Lebert and Benjamin Bacq-Labreuil and Mark P. M. Dean and Kari Ruotsalainen and Alessandro Nicolaou and Simo Huotari and Ikuya Yamada and Hajime Yamamoto and Masaki Azuma and Nicholas B. Brookes and Flora Yakhou and Hu Miao and David Santos-Cottin and Benjamin Lenz and Silke Biermann and Matteo d'Astuto},
  journal= {arXiv preprint arXiv:2303.04139},
  year   = {2023}
}

Comments

11 pages, 5 figures, 2 tables, small corrections in references. Accepted for publication in Physical Review B (American Physical Society)