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Orbital-Selective High-Temperature Cooper Pairing Developed in the Two-Dimensional Limit

Superconductivity 2022-05-16 v1 Mesoscale and Nanoscale Physics Materials Science Strongly Correlated Electrons

Abstract

The orbital multiplicity in multiband superconductors yields orbital differentiation in normal-state properties, and can lead to orbital-selective spin-fluctuation Cooper pairing. This phenomenon has become increasingly pivotal in clarifying the pairing 'enigma' particularly for multiband high-temperature superconductors. In one-unit-cell (1-UC) FeSe/SrTiO3, the thinnest and highest-Tc member of iron-based superconductors, the standard electron-hole Fermi pocket nesting scenario is apparently not applicable since the Gamma-centered hole pockets are absent, so the actual pairing mechanism is the subject of intense debate. Here, by measuring high-resolution Bogoliubov quasiparticle interference, we report observations of highly anisotropic magnetic Cooper pairing in 1-UC FeSe. From a theoretical point of view, it is important to incorporate effects of electronic correlations within a spin-fluctuation pairing calculation, where the dxy orbital becomes coherence-suppressed. The resulting pairing gap is compatible with the experimental findings, which suggests that high-Tc Cooper pairing with orbital selectivity applies to 1-UC FeSe. Our findings imply the general existence of orbital selectivity in iron-based superconductors and the universal importance of electron correlations in high-Tc superconductors.

Keywords

Cite

@article{arxiv.2112.00383,
  title  = {Orbital-Selective High-Temperature Cooper Pairing Developed in the Two-Dimensional Limit},
  author = {Chaofei Liu and Andreas Kreisel and Shan Zhong and Yu Li and Brian M. Andersen and P. J. Hirschfeld and Jian Wang},
  journal= {arXiv preprint arXiv:2112.00383},
  year   = {2022}
}
R2 v1 2026-06-24T07:59:22.088Z