The modern expressions for polarization ¶ and orbital magnetization \M are \k-space integrals. But a genuine bulk property should also be expressible in \r-space, as unambiguous function of the ground-state density matrix, "nearsighted" in insulators, independently of the boundary conditions---either periodic or open. While ¶---owing to its "quantum" indeterminacy---is {\it not} a bulk property in this sense, \M is. We provide its \r-space expression for any insulator, even with nonzero Chern invariant. Simulations on a model Hamiltonian validate our theory.
@article{arxiv.1301.6275,
title = {Orbital Magnetization as a Local Property},
author = {Raffaello Bianco and Raffaele Resta},
journal= {arXiv preprint arXiv:1301.6275},
year = {2013}
}