English

Optical properties of pyrochlore oxide $Pb_{2}Ru_{2}O_{7-{\delta}}$

Materials Science 2009-11-10 v1 Strongly Correlated Electrons

Abstract

We present optical conductivity spectra for Pb2Ru2O7δPb_{2}Ru_{2}O_{7-{\delta}} single crystal at different temperatures. Among reported pyrochlore ruthenates, this compound exhibits metallic behavior in a wide temperature range and has the least resistivity. At low frequencies, the optical spectra show typical Drude responses, but with a knee feature around 1000 \cm. Above 20000 \cm, a broad absorption feature is observed. Our analysis suggests that the low frequency responses can be understood from two Drude components arising from the partially filled Ru t2gt_{2g} bands with different plasma frequencies and scattering rates. The high frequency broad absorption may be contributed by two interband transitions: from occupied Ru t2gt_{2g} states to empty ege_{g} bands and from the fully filled O 2p bands to unoccupied Ru t2gt_{2g} states.

Keywords

Cite

@article{arxiv.cond-mat/0312662,
  title  = {Optical properties of pyrochlore oxide $Pb_{2}Ru_{2}O_{7-{\delta}}$},
  author = {P. Zheng and N. L. Wang and J. L. Luo and R. Jin and D. Mandrus},
  journal= {arXiv preprint arXiv:cond-mat/0312662},
  year   = {2009}
}

Comments

4 pages, 6 figures