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Optical evidence for a magnetically driven structural transition in the spin web $Cu_3TeO_6$

Strongly Correlated Electrons 2012-01-11 v1 Materials Science

Abstract

Cu3TeO6Cu_3TeO_6 is a modest frustrated S=1/2S=1/2 spin system, which undergoes an anti-ferromagnetic transition at TN61T_N\sim61 KK. The anti-ferromagnetic spin alignment in Cu3TeO6Cu_3TeO_6 below TNT_N is supposed to induce a magneto-elastic strain of the lattice. The complete absorption spectrum of Cu3TeO6Cu_3TeO_6 is obtained through Kramers-Kronig transformation of the optical reflectivity, measured from the far-infrared up to the ultraviolet spectral range as a function of temperature (TT). Below T50T^*\sim 50 KK, we find a new mode at 208 cm1cm^{-1}. The spectral weight associated to this additional mode increases as (TT)1/2\propto (T^*-T)^{1/2} with decreasing TT below TT^*. The implication of the optical findings will be discussed in relation to the magnetic phase transition at TNT_N.

Keywords

Cite

@article{arxiv.cond-mat/0510186,
  title  = {Optical evidence for a magnetically driven structural transition in the spin web $Cu_3TeO_6$},
  author = {G. Caimi and L. Degiorgi and H. Berger and L. Forro},
  journal= {arXiv preprint arXiv:cond-mat/0510186},
  year   = {2012}
}

Comments

9 pages, 3 figures

R2 v1 2026-07-22T11:23:44.554Z