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One-shot trajectory learning of open quantum systems dynamics

Quantum Physics 2022-06-28 v2 Chemical Physics

Abstract

Nonadiabatic quantum dynamics are important for understanding light-harvesting processes, but their propagation with traditional methods can be rather expensive. Here we present a one-shot trajectory learning approach that allows to directly make ultra-fast prediction of the entire trajectory of the reduced density matrix for a new set of such simulation parameters as temperature and reorganization energy. The whole 10ps long propagation takes 70 milliseconds as we demonstrate on the comparatively large quantum system, the Fenna-Matthews-Olsen (FMO) complex. Our approach also significantly reduces time and memory requirements for training.

Keywords

Cite

@article{arxiv.2204.12661,
  title  = {One-shot trajectory learning of open quantum systems dynamics},
  author = {Arif Ullah and Pavlo O. Dral},
  journal= {arXiv preprint arXiv:2204.12661},
  year   = {2022}
}
R2 v1 2026-06-24T10:59:43.848Z