English

On the "Causality Paradox" of Time-Dependent Density Functional Theory

Materials Science 2009-11-13 v1

Abstract

I show that the so-called causality paradox of time-dependent density functional theory arises from an incorrect formulation of the variational principle for the time evolution of the density. The correct formulation not only resolves the paradox in real time, but also leads to a new expression for the causal exchange-correlation kernel in terms of Berry curvature. Furthermore, I show that all the results that were previously derived from symmetries of the action functional remain valid in the present formulation. Finally, I develop a model functional theory which explicitly demonstrates the workings of the new formulation.

Keywords

Cite

@article{arxiv.0803.2727,
  title  = {On the "Causality Paradox" of Time-Dependent Density Functional Theory},
  author = {G. Vignale},
  journal= {arXiv preprint arXiv:0803.2727},
  year   = {2009}
}

Comments

21 pages

R2 v1 2026-06-21T10:22:37.513Z