Understanding how renormalized quasiparticles emerge in strongly correlated electron materials provides a challenge for both experiment and theory. It has been predicted that distinctive spin and orbital screening mechanisms drive this process in multiorbital materials with strong Coulomb and Hund's interactions. Here, we provide the experimental evidence of both mechanisms from angle-resolved photoemission spectroscopy on RbFe2As2. We observe that the emergence of low-energy Fe 3dxy quasiparticles below 90K is tied to spin screening. A second process changes the spectral weight at high energies up to room temperature. Supported by theoretical calculations we attribute it to orbital screening of Fe 3d atomic excitations. These two cascading screening processes drive the temperature evolution from a bad metal to a correlated Fermi liquid.
@article{arxiv.2503.06314,
title = {Observation of Two Cascading Screening Processes in an Iron-based Superconductor},
author = {Ming-Hua Chang and Steffen Backes and Donghui Lu and Nicolas Gauthier and Makoto Hashimoto and Guan-Yu Chen and Hai-Hu Wen and Sung-Kwan Mo and Zhi-Xun Shen and Roser Valenti and Heike Pfau},
journal= {arXiv preprint arXiv:2503.06314},
year = {2025}
}