English

Observation of correlation-driven topological transport and robust ferromagnetism in 2D CrS$_2$

Materials Science 2026-07-26 v1 Strongly Correlated Electrons

Abstract

The realization of correlated layered magnets hosting robust ferromagnetism with emergent topological transport remains a key challenge in quantum materials. Here we report the first catalyst-free chemical vapour deposition growth of layered 1T-CrS2_2, establishing a highly stable vdWs ferromagnet with an out-of-plane easy-axis anisotropy and a Curie temperature above room temperature. Transport measurements reveal a semimetal--insulator crossover near 80 K and pronounced negative magnetoresistance up to 350 K. A topological Hall effect emerges below 30 K, a rare signature of correlated transport in layered transition-metal dichalcogenide ferromagnets. First-principles calculations show that spin--orbit coupling gaps Dirac-like crossings, while electronic correlations reconstruct the Fermi surface by suppressing electron pockets and reducing the carrier density, enhancing momentum-dependent out-of-plane spin polarization. Magnetic measurements, supported by Heisenberg exchange calculations, reveal strong nearest-neighbour ferromagnetic exchange that stabilizes long-range ferromagnetism. Our results establish 1T-CrS2_2 as a rare correlated 3dd layered ferromagnet in which electronic correlations and spin--orbit coupling cooperatively drive emergent topological transport.

Keywords

Cite

@article{arxiv.2607.23625,
  title  = {Observation of correlation-driven topological transport and robust ferromagnetism in 2D CrS$_2$},
  author = {Sk Md Obaidulla and M. Nur Hasan and Dayal Das and Rafiqul Alam and Antonio Supina and Muhammad Awais Aslam and Sherif Kamal and Iva Šarić Jankovic and Aleksandar Matkovic and Christian Teichert and Atindra Nath Pal and Heike C. Herper and Marko Kralj},
  journal= {arXiv preprint arXiv:2607.23625},
  year   = {2026}
}

Comments

10 Pages, 4 figures and additional supplementary information