English

Novel approach to description of quantum magnets with large singe-ion easy-plane anisotropy

Strongly Correlated Electrons 2012-06-01 v1

Abstract

We introduce a new representation of an integer spin SS via bosonic operators which is useful in describing the paramagnetic phase and transitions to magnetically ordered phases in magnetic systems with large single-ion easy-plane anisotropy DD. Considering the exchange interaction between spins as a perturbation and using the diagram technique we derive the elementary excitation spectrum and the ground state energy in the third order of the perturbation theory. In the special case of S=1 we obtain these expressions also using simpler spin representations some of which were introduced before. Comparison with results of previous numerical studies of 2D systems with S=1 demonstrates that our approach works better than other analytical methods applied before for such systems. We apply our results for the elementary excitation spectrum analysis obtained experimentally in NiCl2\rm NiCl_2-4SC(NH2)2\rm 4SC(NH_2)_2 (DTN). It is demonstrated that a set of model parameters (exchange constants and DD) which has been used for DTN so far describes badly the experimentally obtained spectrum. A new set of parameters is proposed using which we fit the spectrum and values of two critical fields of DTN.

Keywords

Cite

@article{arxiv.1105.1077,
  title  = {Novel approach to description of quantum magnets with large singe-ion easy-plane anisotropy},
  author = {Alexey V Sizanov and Arseny V Syromyatnikov},
  journal= {arXiv preprint arXiv:1105.1077},
  year   = {2012}
}

Comments

15 pages, 8 figures