English

Nonequilibrium GW+EDMFT: Antiscreening and inverted populations from nonlocal correlations

Strongly Correlated Electrons 2017-06-21 v2

Abstract

We study the dynamics of screening in photo-doped Mott insulators with long-ranged interactions using a nonequilibrium implementation of the GWGW plus extended dynamical mean field theory (GWGW+EDMFT) formalism. Our study demonstrates that the complex interplay of the injected carriers with bosonic degrees of freedom (charge fluctuations) can result in long-lived transient states with properties that are distinctly different from those of thermal equilibrium states. Systems with strong nonlocal interactions are found to exhibit a self-sustained population inversion of the doublons and holes. This population inversion leads to low-energy antiscreening which can be detected in time-resolved electron-energy loss spectra.

Keywords

Cite

@article{arxiv.1702.04952,
  title  = {Nonequilibrium GW+EDMFT: Antiscreening and inverted populations from nonlocal correlations},
  author = {Denis Golez and Lewin Boehnke and Hugo Strand and Martin Eckstein and Philipp Werner},
  journal= {arXiv preprint arXiv:1702.04952},
  year   = {2017}
}