English

Non-equilbrium Dynamics in Amorphous Si_3B_3N_7

Statistical Mechanics 2007-05-23 v1 Disordered Systems and Neural Networks

Abstract

We present extensive numerical investigations of the structural relaxation dynamics of a realistic model of the amorphous high-temperature ceramic a-Si3_3B3_3N7_7, probing the mean square displacement (MSD) of the atoms, the bond survival probability (BSP), the average energy, the specific heat, and the two-point energy average. Combining the information from these different sources, we identify a transition temperature Tc2000T_c \approx 2000 K below which the system is no longer ergodic and physical quantities observed over a time tobst_{obs} show a systematic parametric dependence on the waiting time twt_w, or age, elapsed after the quench. The aging dynamics 'stiffens' as the system becomes older, which is similar to the behavior of highly idealized models such as Ising spin-glasses and Lennard-Jones glasses.

Keywords

Cite

@article{arxiv.cond-mat/0504384,
  title  = {Non-equilbrium Dynamics in Amorphous Si_3B_3N_7},
  author = {A. Hannemann and J. C. Schön and M. Jansen and P. Sibani},
  journal= {arXiv preprint arXiv:cond-mat/0504384},
  year   = {2007}
}

Comments

Journal of Phys. Chem.B in press.Extended version of paper cond-mat/0212245