Non-collinear magnetism in Al-Mn topologically disordered systems
Abstract
We have performed the first ab-initio calculations of a possible complex non-collinear magnetic structure in aluminium-rich Al-Mn liquids within the real-space tight-binding LMTO method. In our previous work we predicted the existence of large magnetic moments in Al-Mn liquids [A.M. Bratkovsky, A.V. Smirnov, D. N. Manh, and A. Pasturel, \prb {\bf 52}, 3056 (1995)] which has been very recently confirmed experimentally. Our present calculations show that there is a strong tendency for the moments on Mn to have a non-collinear (random) order retaining their large value of about 3~. The d-electrons on Mn demonstrate a pronounced non-rigid band behaviour which cannot be reproduced within a simple Stoner picture. The origin of the magnetism in these systems is a topological disorder which drives the moments formation and frustrates their directions in the liquid phase.
Keywords
Cite
@article{arxiv.cond-mat/9512013,
title = {Non-collinear magnetism in Al-Mn topologically disordered systems},
author = {A. V. Smirnov and A. M. Bratkovsky},
journal= {arXiv preprint arXiv:cond-mat/9512013},
year = {2009}
}
Comments
10 pages, RevTex 3.0, 24kb. 3 PS figures available on request from [email protected] The work has been presented at ERC ``Electronic Structire of Solids'' (Lunteren, The Netherlands, 9-14 September 1995)