English

NMR Evidence of Antiferromagnetic Spin Fluctuations in Nd$_{0.85}$Sr$_{0.15}$NiO$_2$

Superconductivity 2021-05-31 v2 Strongly Correlated Electrons

Abstract

Despite the recent discovery of superconductivity in Nd1x_{1-x}Srx_{x}NiO2_2 thin films, the absence of superconductivity and antiferromagnetism in their bulk materials remain a puzzle. Here we report the 1^{1}H NMR measurements on powdered Nd0.85_{0.85}Sr0.15_{0.15}NiO2_2 samples by taking advantage of the enriched proton concentration after hydrogen annealing. We find a large full width at half maximum of the spectrum, which keeps increasing with decreasing the temperature and exhibits an upturn behavior at low temperatures. The spin-lattice relaxation rate 1/1T11/^{1}T_1 is strongly enhanced when lowering the temperature, developing a broad peak at about 40 K, then decreases following a spin-wave-like behavior 1/1T1T21/^{1}T_1{\sim}T^2 at lower temperatures. These results evidence a short-range glassy antiferromagnetic ordering of magnetic moments below 40 K and dominant antiferromagnetic fluctuations extending to much higher temperatures. Our findings reveal the strong electron correlations in bulk Nd0.85_{0.85}Sr0.15_{0.15}NiO2_2, and shed light on the mechanism of superconductivity observed in films of nickelates.

Keywords

Cite

@article{arxiv.2011.09610,
  title  = {NMR Evidence of Antiferromagnetic Spin Fluctuations in Nd$_{0.85}$Sr$_{0.15}$NiO$_2$},
  author = {Yi Cui and C. Li and Q. Li and Xiyu Zhu and Z. Hu and Yi-feng Yang and J. S. Zhang and Rong Yu and Hai-Hu Wen and Weiqiang Yu},
  journal= {arXiv preprint arXiv:2011.09610},
  year   = {2021}
}

Comments

6 pages, 4 figures