English

Multipolar spin liquid in an exactly solvable model for $j_\mathrm{eff} = \frac{3}{2}$ moments

Strongly Correlated Electrons 2023-10-17 v2

Abstract

We study an exactly solvable model with bond-directional quadrupolar and octupolar interactions between spin-orbital entangled jeff=32j_{\mathrm{eff}} = \frac{3}{2} moments on the honeycomb lattice. We show that this model features a multipolar spin liquid phase with gapless fermionic excitations. In the presence of perturbations that break time-reversal and rotation symmetries, we find Abelian and non-Abelian topological phases in which the Chern number evaluates to 00, ±1\pm 1, and ±2\pm 2. We also investigate quantum phase transitions out of the multipolar spin liquid using a parton mean-field approach and orbital wave theory. In the regime of strong integrability-breaking interactions, the multipolar spin liquid gives way to ferroquadrupolar-vortex and antiferro-octupolar ordered phases that harbor a hidden spin-12\frac{1}{2} Kitaev spin liquid. Our work unveils mechanisms for unusual multipolar orders and quantum spin liquids in Mott insulators with strong spin-orbit coupling.

Keywords

Cite

@article{arxiv.2306.08624,
  title  = {Multipolar spin liquid in an exactly solvable model for $j_\mathrm{eff} = \frac{3}{2}$ moments},
  author = {Vanuildo S. de Carvalho and Hermann Freire and Rodrigo G. Pereira},
  journal= {arXiv preprint arXiv:2306.08624},
  year   = {2023}
}

Comments

14 pages, 9 figures