English

Multi-time Formulation of Matsubara Dynamics

Chemical Physics 2019-09-04 v1

Abstract

Matsubara dynamics has recently emerged as the most general form of a quantum-Boltzmann-conserving classical dynamics theory for the calculation of single-time correlation functions. Here, we present a generalization of Matsubara dynamics for the evaluation of multi-time correlation functions. We show that the Matsubara approximation can also be used to approximate the two-time symmetrized double Kubo transformed correlation function. By a straightforward extension of these ideas to the multi-time realm, a multi-time Matsubara dynamics approximation can be obtained for the multi-time fully symmetrized Kubo transformed correlation function. Although not a practical method, due to the presence of a phase-term, this multi-time formulation of Matsubara dynamics represents a benchmark theory for future development of Boltzmann preserving semi-classical approximations to general higher order multi-time correlation functions.

Cite

@article{arxiv.1810.01840,
  title  = {Multi-time Formulation of Matsubara Dynamics},
  author = {Kenneth A. Jung and Pablo E. Videla and Victor S. Batista},
  journal= {arXiv preprint arXiv:1810.01840},
  year   = {2019}
}
R2 v1 2026-06-23T04:27:30.791Z