English

Molecular ion trap-depletion spectroscopy of BaCl$^+$

Atomic Physics 2015-05-27 v1 Chemical Physics

Abstract

We demonstrate a simple technique for molecular ion spectroscopy. BaCl+^+ molecular ions are trapped in a linear Paul trap in the presence of a room-temperature He buffer gas and photodissociated by driving an electronic transition from the ground X1Σ+^1\Sigma^+ state to the repulsive wall of the A1Π^1\Pi state. The photodissociation spectrum is recorded by monitoring the induced trap loss of BaCl+^+ ions as a function of excitation wavelength. Accurate molecular potentials and spectroscopic constants are determined. Comparison of the theoretical photodissociation cross-sections with the measurement shows excellent agreement. This study represents the first spectroscopic data for BaCl+^+ and an important step towards the production of ultracold ground-state molecular ions.

Keywords

Cite

@article{arxiv.1101.4259,
  title  = {Molecular ion trap-depletion spectroscopy of BaCl$^+$},
  author = {Kuang Chen and Steven J. Schowalter and Svetlana Kotochigova and Alexander Petrov and Wade G. Rellergert and Scott T. Sullivan and Eric R. Hudson},
  journal= {arXiv preprint arXiv:1101.4259},
  year   = {2015}
}

Comments

5 pages, 5 figures