We investigate twisted double bilayer graphene (TDBG), a four-layer system composed of two AB-stacked graphene bilayers rotated with respect to each other by a small angle. Our ab initio band structure calculations reveal a considerable energy gap at the charge point neutrality that we assign to the intrinsic symmetric polarization (ISP). We then introduce the ISP effect into the tight-binding parameterization and perform calculations on TDBG models that include lattice relaxation effects down to very small twist angles. We identify a narrow region around the magic angle θ∘=1.3∘ characterized by a manifold of remarkably flat bands gapped out from other states even without external electric fields. To understand the fundamental origin of the magic angle in TDBG, we construct a continuum model that points to a hidden mathematical link to the twisted bilayer graphene (TBG) model, thus indicating that the band flattening is a fundamental feature of TDBG, and is not a result of external fields.
@article{arxiv.1906.00623,
title = {Moir\'e Flat Bands in Twisted Double Bilayer Graphene},
author = {Fatemeh Haddadi and QuanSheng Wu and Alex J. Kruchkov and Oleg V. Yazyev},
journal= {arXiv preprint arXiv:1906.00623},
year = {2020}
}