Measurement of spin coherence using Raman scattering

Ramsey interferometry provides a natural way to determine the coherence time of most qubit systems. Recent experiments on quantum dots however, demonstrated that dynamical nuclear spin polarization can strongly influence the measurement process, making it difficult to extract the $T_2^*$ coherence time using optical Ramsey pulses. Here, we demonstrate an alternative method for spin coherence measurement that is based on first-order coherence of photons generated in spin-flip Raman scattering. We show that if a quantum emitter is driven by a weak monochromatic laser, Raman coherence is determined exclusively by spin coherence, allowing for a direct determination of spin $T_2^*$ time. When combined with coherence measurements on Rayleigh scattered photons, our technique enables us to identify coherent and incoherent contributions to resonance fluorescence, and to minimize the latter. We verify the validity of our technique by comparing our results to those determined from Ramsey interferometry for electron and heavy-hole spins.