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Many-body large polaron optical conductivity in SrTi$_{1-x}$Nb$_x$O$_3$

Strongly Correlated Electrons 2015-05-18 v1 Materials Science

Abstract

Recent experimental data on the optical conductivity of niobium doped SrTiO3_{3} are interpreted in terms of a gas of large polarons with effective coupling constant αeff2\alpha_{eff}\approx2. The {theoretical approach takes into account} many-body effects, the electron-phonon interaction with multiple LO-phonon branches, and the degeneracy and the anisotropy of the Ti t2g_{2g} conduction band. {Based on the Fr\"{o}hlich interaction, the many-body large-polaron theory} provides an interpretation for the essential characteristics, except -- interestingly -- for the unexpectedly large intensity of a peak at 130\sim130 meV, of the observed optical conductivity spectra of SrTi1x_{1-x}Nbx_{x}O3_{3} \textit{without} any adjustment of material parameters.

Keywords

Cite

@article{arxiv.1003.1003,
  title  = {Many-body large polaron optical conductivity in SrTi$_{1-x}$Nb$_x$O$_3$},
  author = {J. T. Devreese and S. N. Klimin and J. L. M. van Mechelen and D. van der Marel},
  journal= {arXiv preprint arXiv:1003.1003},
  year   = {2015}
}

Comments

to appear in Phys. Rev. B