English

Magnon-magnon interactions in the Spin-Peierls compound CuGeO_3

Strongly Correlated Electrons 2009-10-28 v1

Abstract

In a magnetic substance the gap in the Raman spectrum, Delta_R, is approximatively twice the value of the neutron scattering gap, Delta_S, if the the magnetic excitations (magnons) are only weakly interacting. But for CuGeO_3 the experimentally observed ratio Delta_R/Delta_S is approximatively 1.49-1.78, indicating attractive magnon-magnon interactions in the quasi-1D Spin-Peierls compound CuGe_3. We present numerical estimates for Delta_R/Delta_S from exact diagonalization studies for finite chains and find agreement with experiment for intermediate values of the frustration parameter alpha. An analysis of the numerical Raman intensity leads us to postulate a continuum of two-magnon bound states in the Spin-Peierls phase. We discuss in detail the numerical method used, the dependence of the results on the model parameters and a novel matrix-element effect due to the dimerization of the Raman-operator in the Spin-Peierls phase.

Keywords

Cite

@article{arxiv.cond-mat/9612101,
  title  = {Magnon-magnon interactions in the Spin-Peierls compound CuGeO_3},
  author = {C. Gros and W. Wenzel and A. Fledderjohann and P. Lemmens and M. Fischer and G. Güntherodt and M. Weiden and C. Geibel and F. Steglich},
  journal= {arXiv preprint arXiv:cond-mat/9612101},
  year   = {2009}
}

Comments

submitted to PRB, Phys. Rev. B, in press