English

Magnetostriction and magnetostructural domains in CoTiO$_3$

Strongly Correlated Electrons 2021-09-27 v1 Materials Science

Abstract

We report the magnetostrictive length changes of CoTiO3_3 studied by means of high-resolution dilatometry in magnetic fields (BB) up to 15~T. In the long-range antiferromagnetically ordered phase below TNT_N = 38~K, the easy-plane type spin structure undergoes a spin-reorientation transition in the abab plane in magnetic fields Bab2B || ab \approx 2~T. We observe pronounced length changes driven by external magnetic field in this field region indicating significant magnetoelastic coupling in CoTiO3_3. Specifically, we observe anisotropic deformation of the lattice for fields applied in the abab plane. While, for B2B \lesssim 2~T, in-plane magnetostriction shows that the lattice expands (contracts) parallel (perpendicular) to the field direction, the opposite behaviour appear at higher fields. Furthermore, there are remarkable effects of slight changes in the applied uniaxial pressure on the magnetostrictive response of CoTiO3_3 persisting to temperatures well above TNT_N. The data evidence the presence of magnetic domains below TNT_N as well as of structural ones in CoTiO3_3. The presence of magnetic domains in the spin ordered phase is further evidenced by an additional 3-fold magnetic anisotropy appearing below TNT_N. We discuss the effects of rotational magnetic domains on isothermal magnetization and magnetostriction and interpret our results on the basis of a multi-domain phenomenological model.

Keywords

Cite

@article{arxiv.2109.11923,
  title  = {Magnetostriction and magnetostructural domains in CoTiO$_3$},
  author = {K. Dey and M. Hoffmann and R. Klingeler},
  journal= {arXiv preprint arXiv:2109.11923},
  year   = {2021}
}
R2 v1 2026-06-24T06:17:41.238Z