English

Magnetoelastic phenomena in antiferromagnetic uranium intermetallics: the $\mathrm{UAu_{2}Si_{2}}$ case

Strongly Correlated Electrons 2018-12-05 v2

Abstract

Thermal expansion, magnetostriction and magnetization measurements under magnetic field and hydrostatic pressure were performed on a UAu2Si2\mathrm{UAu_{2}Si_{2}} single crystal. They revealed a large anisotropy of magnetoelastic properties manifested by prominent length changes leading to a collapse of the unit-cell volume accompanied by breaking the fourfold symmetry (similar to that in URu2Si2\mathrm{URu_{2}Si_{2}} in the hidden-order state) in the antiferromagnetic state as consequences of strong magnetoelastic coupling. The magnetostriction curves measured at higher temperatures confirm a bulk character of the 50 K weak ferromagnetic phase. The large positive pressure change of the ordering temperature predicted from Ehrenfest relation contradicts the more than an order of magnitude smaller pressure dependence observed by the magnetization and specific heat measured under hydrostatic pressure. A comprehensive magnetic phase diagram of UAu2Si2\mathrm{UAu_{2}Si_{2}} in magnetic field applied along the cc axis is presented. The ground-state antiferromagnetic phase is suppressed by a field-induced metamagnetic transition that changes its character from the second to the first order at the tricritical point.

Keywords

Cite

@article{arxiv.1804.11180,
  title  = {Magnetoelastic phenomena in antiferromagnetic uranium intermetallics: the $\mathrm{UAu_{2}Si_{2}}$ case},
  author = {M. Vališka and H. Saito and T. Yanagisawa and Ch. Tabata and H. Amitsuka and K. Uhlířová and J. Prokleška and P. Proschek and J. Valenta and M. Míšek and D. I. Gorbunov and J. Wosnitza and V. Sechovský},
  journal= {arXiv preprint arXiv:1804.11180},
  year   = {2018}
}