English

Magneto-Dielectric Behavior in $La_{0.53}Ca_{0.47}MnO_{3}$

Materials Science 2017-07-26 v2

Abstract

We prospect magneto-dielectricity in La0.53Ca0.47MnO3La_{0.53}Ca_{0.47}MnO_{3} across its paramagnetic (PMI) to ferromagnetic (FMM) isostructural transition at TC253KT_{C} \sim 253K, by magnetic ((M)(M)), caloric ((W)(W)), dielectric ((ϵ)(\epsilon')), magneto-resistive (MR), and magneto-capacitance (MC) investigations. Skew-broadened first-order transition character is confirmed via heating/cooling hystereses in (M)(T)(M)(T) and (W)(T)(W)(T), with superheating temperature TT** almost next to TCT_C and supercooling temperature TT* exhibiting kinetics. Above TCT_C, linearly-related MC and MR reflect purely magneto-resistance effect. Near TCT_C, the high-frequency MC(5T) much exceeds the magneto-losses, and is uncorrelated with dc MR(5T) in the FM-ordered state. The intrinsic magneto-dielectricity manifest below TCT_C and above ~kHz is traced to an intra-granular Maxwell-Wagner-type effect at the interface-region of PMI-FMM phase-coexistence.

Keywords

Cite

@article{arxiv.1408.6640,
  title  = {Magneto-Dielectric Behavior in $La_{0.53}Ca_{0.47}MnO_{3}$},
  author = {Suchita Pandey and Jitender Kumar and A. M. Awasthi},
  journal= {arXiv preprint arXiv:1408.6640},
  year   = {2017}
}

Comments

16 pages, 5 figures, and 39 references