English

Magnetic short and long range order in PbFe$_{1/2}$Ta$_{1/2}$O$_{3}$

Strongly Correlated Electrons 2014-08-20 v2

Abstract

PbFe1/2_{1/2}Ta1/2_{1/2}O3_{3} (PFT) belongs to the family of PbBx'_{x}B"1x"_{1-x}O3_{3} which have inherent chemical disorder at the B-site. Due to this disorder, a complex magnetic phase diagram is expected in the material. In this paper, we report experimental results of magnetic properties in PFT through macroscopic characterization, neutron scattering and M\"{o}ssbauer spectroscopy techniques. With these results we show for the first time that PbFe1/2_{1/2}Ta1/2_{1/2}O3_{3} behaves very similar to PbFe1/2_{1/2}Nb1/2_{1/2}O3_{3}, i.e, it undergoes AF transition at 153 K and has a spinglass transition at 10 K, below which the antiferromagnetism coexists with spinglass. We suggest that the mechanism which is responsible for such a non-trivial ground state can be explained by a speromagnet-like spin arrangement similar to the one proposed for PbFe1/2_{1/2}Nb1/2_{1/2}O3_{3}.

Keywords

Cite

@article{arxiv.1402.2914,
  title  = {Magnetic short and long range order in PbFe$_{1/2}$Ta$_{1/2}$O$_{3}$},
  author = {S. Chillal and S. N. Gvasaliya and D. Schroeter and M. Kraken and F. J. Litterst and T. A. Shaplygina and S. G. Lushnikov and A. Zheludev},
  journal= {arXiv preprint arXiv:1402.2914},
  year   = {2014}
}

Comments

7 pages, 8 figures