English

Magnetic Polarons Enable Exceptional Magnetocaloric Response

Materials Science 2026-04-22 v1

Abstract

Magnetocaloric materials are typically limited by a trade-off between magnetic entropy and field responsiveness. Here we show that magnetic polarons provide an intermediate regime that mitigates this constraint and enables an exceptional magnetocaloric response. Using EuB6_6 as a model system, we combine thermodynamic and magnetic measurements to demonstrate that nanoscale ferromagnetic clusters emerging near the Curie temperature strongly enhance the field-induced entropy collapse. These clusters possess large effective moments that respond efficiently to applied fields while retaining substantial entropy due to their small size and dynamic fluctuations. As a result, EuB6_6 exhibits a giant cryogenic magnetocaloric response, with both large isothermal entropy change and adiabatic temperature change in the technologically important 10-40 K range. Our results identify magnetic polarons as an underexplored route for optimizing magnetocaloric performance and establish an intermediate magnetic length scale as a design principle for high-performance cryogenic cooling materials.

Keywords

Cite

@article{arxiv.2604.18938,
  title  = {Magnetic Polarons Enable Exceptional Magnetocaloric Response},
  author = {Joshua Ancheta and Caeli Benyacko and Fanghao Zhang and Stephen D. Wilson and Bolin Liao},
  journal= {arXiv preprint arXiv:2604.18938},
  year   = {2026}
}
R2 v1 2026-07-01T12:27:26.889Z