We investigate the magnetic properties of nano-holes (NHs) patterned in graphene using first principles calculations. We show that superlattices consisting of a periodic array of NHs form a new family of 2D crystalline "bulk" magnets whose collective magnetic behavior is governed by inter-NH spin-spin interaction. They exhibit long-range magnetic order well above room temperature. Furthermore, magnetic semiconductors can be made by doping magnetic NHs into semiconducting NH superlattices. Our findings offer a new material system for fundamental studies of spin-spin interaction and magnetic ordering in low dimensions, and open up the exciting opportunities of making engineered magnetic materials for storage media and spintronics applications.
@article{arxiv.0803.2660,
title = {Magnetic Graphene Nanohole Superlattices},
author = {Decai Yu and Elizabeth M. Lupton and Miao Liu and Wei Liu and Feng Liu},
journal= {arXiv preprint arXiv:0803.2660},
year = {2010}
}