English

Magnetic dipole transitions in the OH $A\,^2\Sigma^+ \leftarrow X\,^2\Pi$ system

Chemical Physics 2012-08-27 v1 Quantum Physics

Abstract

We report on the observation of magnetic dipole allowed transitions in the well-characterized A2Σ+X2ΠA\,^2\Sigma^+ - X\,^2\Pi band system of the OH radical. A Stark decelerator in combination with microwave Rabi spectroscopy is used to control the populations in selected hyperfine levels of both Λ\Lambda-doublet components of the X2Π3/2,v=0,J=3/2X\,^2\Pi_{3/2},v=0,J=3/2 ground state. Theoretical calculations presented in this paper predict that the magnetic dipole transitions in the ν=1ν=0\nu'=1 \leftarrow \nu=0 band are weaker than the electric dipole transitions by a factor of 2.58×1032.58\times 10^3 only, i.e., much less than commonly believed. Our experimental data confirm this prediction.

Keywords

Cite

@article{arxiv.1208.4939,
  title  = {Magnetic dipole transitions in the OH $A\,^2\Sigma^+ \leftarrow X\,^2\Pi$ system},
  author = {Moritz Kirste and Xingan Wang and Gerard Meijer and Koos B. Gubbels and Ad van der Avoird and Gerrit C. Groenenboom and Sebastiaan Y. T. van de Meerakker},
  journal= {arXiv preprint arXiv:1208.4939},
  year   = {2012}
}