English

"Madelung model" prediction for dependence of lattice parameter on nanocrystal size

Materials Science 2009-11-07 v1

Abstract

The competition between the long range Coulomb attractive and the short range repulsive interaction in ionic nanocrystals creates an effective negative pressure, which causes the lattice parameter a to increase with decreasing nanoparticle size d. A simple ``Madelung model'' is used to predict the dependence of the lattice parameter for CeO2 and BaTiO3 on d, delta a/a = alpha/d, for alpha = 0.22 A and 0.18 A respectively. The model predictions are compared with experimental results.

Keywords

Cite

@article{arxiv.cond-mat/0208048,
  title  = {"Madelung model" prediction for dependence of lattice parameter on nanocrystal size},
  author = {Vasili Perebeinos and Siu-Wai Chan and Feng Zhang},
  journal= {arXiv preprint arXiv:cond-mat/0208048},
  year   = {2009}
}

Comments

5 pages, 2 figures